Continuous ageing trajectory representations for knee-aware lifetime prediction of lithium-ion batteries across heterogeneous dataset

Abstract

Accurate assessment of lithium-ion battery ageing is challenged by cell-to-cell variability, heterogeneous cycling protocols, and limited transferability of data-driven models across datasets. In particular, robust identification of degradation transitions, such as the knee point, and reliable early-life prediction of remaining useful life (RUL) remain open problems. This study proposes a unified framework for battery ageing analysis based on continuous representations of voltage-capacity and capacity-cycle trajectories learned from heterogeneous public datasets (NASA, CALCE, ISU-ILCC). The continuous formulation enables consistent extraction of degradation descriptors, including curvature, plateau length and knee-related metrics, while reducing sensitivity to dataset-specific discretisation. Across more than 250 cells, statistically significant correlations between knee onset and end-of-life (Pearson 0.75-0.84) are observed. Additional early-life analysis confirms that knee-related features retain predictive value when estimated from partial trajectories. Early-life models provide increasingly stable RUL predictions as the number of observed cycles increases, with meaningful predictive performance emerging within the first 5-20 cycles and remain robust under cross-dataset domain shift. The framework integrates continuous modelling, feature extraction and uncertainty-aware prediction, providing an interpretable and dataset-consistent approach demonstrating robustness across heterogeneous dataset types. Compared with conventional discrete or feature-based methods, the proposed representation reduces sensitivity to sampling resolution and improves cross-dataset consistency. The study is limited to laboratory-scale datasets and capacity-based end-of-life definitions.